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1.
Environ Sci Technol ; 58(11): 4948-4956, 2024 Mar 19.
Artículo en Inglés | MEDLINE | ID: mdl-38445593

RESUMEN

Methane emissions from the oil and gas supply chain can be intermittent, posing challenges for monitoring and mitigation efforts. This study examines shallow water facilities in the US Gulf of Mexico with repeat atmospheric observations to evaluate temporal variation in site-specific methane emissions. We combine new and previous observations to develop a longitudinal study, spanning from days to months to almost five years, evaluating the emissions behavior of sites over time. We also define and determine the chance of subsequent detection (CSD): the likelihood that an emitting site will be observed emitting again. The average emitting central hub in the Gulf has a 74% CSD at any time interval. Eight facilities contribute 50% of total emissions and are over 80% persistent with a 96% CSD above 100 kg/h and 46% persistent with a 42% CSD above 1000 kg/h, indicating that large emissions are persistent at certain sites. Forward-looking infrared (FLIR) footage shows many of these sites exhibiting cold venting. This suggests that for offshore, a low sampling frequency over large spatial coverage can capture typical site emissions behavior and identify targets for mitigation. We further demonstrate the preliminary use of space-based observations to monitor offshore emissions over time.


Asunto(s)
Contaminantes Atmosféricos , Metano , Metano/análisis , Golfo de México , Estudios Longitudinales , Contaminantes Atmosféricos/análisis , Probabilidad , Gas Natural
2.
Sci Adv ; 8(32): eabn9683, 2022 Aug 12.
Artículo en Inglés | MEDLINE | ID: mdl-35947659

RESUMEN

As atmospheric methane concentrations increase at record pace, it is critical to identify individual emission sources with high potential for mitigation. Here, we leverage the synergy between satellite instruments with different spatiotemporal coverage and resolution to detect and quantify emissions from individual landfills. We use the global surveying Tropospheric Monitoring Instrument (TROPOMI) to identify large emission hot spots and then zoom in with high-resolution target-mode observations from the GHGSat instrument suite to identify the responsible facilities and characterize their emissions. Using this approach, we detect and analyze strongly emitting landfills (3 to 29 t hour-1) in Buenos Aires, Delhi, Lahore, and Mumbai. Using TROPOMI data in an inversion, we find that city-level emissions are 1.4 to 2.6 times larger than reported in commonly used emission inventories and that the landfills contribute 6 to 50% of those emissions. Our work demonstrates how complementary satellites enable global detection, identification, and monitoring of methane superemitters at the facility level.

3.
Environ Sci Technol ; 54(16): 10246-10253, 2020 08 18.
Artículo en Inglés | MEDLINE | ID: mdl-32672947

RESUMEN

Satellite observations of atmospheric methane plumes offer a means for global mapping of methane point sources. Here we use the GHGSat-D satellite instrument with 50 m effective spatial resolution and 9-18% single-pass column precision to quantify mean source rates for three coal mine vents (San Juan, United States; Appin, Australia; and Bulianta, China) over a two-year period (2016-2018). This involves averaging wind-rotated observations from 14 to 24 overpasses to achieve satisfactory signal-to-noise. Our wind rotation method optimizes the wind direction information for individual plumes to account for error in meteorological databases. We derive source rates from the time-averaged plumes using integrated mass enhancement (IME) and cross-sectional flux (CSF) methods calibrated with large eddy simulations. We find time-averaged source rates ranging from 2320 to 5850 kg h-1 for the three coal mine vents, with 40-45% precision (1σ), and generally consistent with previous estimates. The IME and CSF methods agree within 15%. Our results demonstrate the potential of space-based monitoring for annual reporting of methane emissions from point sources and suggest that future satellite instruments with similar pixel resolution but better precision should be able to constrain a wide range of point sources.


Asunto(s)
Contaminantes Atmosféricos , Metano , Contaminantes Atmosféricos/análisis , Australia , China , Carbón Mineral , Estudios Transversales , Monitoreo del Ambiente , Metano/análisis
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